I use both bone and metal needles for sewing. Bone isn't all that sharp, but is surprisingly tough. It's much harder to make a *fine* bone needle than a metal one, though.
I've never tried (deliberate) skin piercing with needles, but going by how often I've done it accidentally I'd say metal has a distinct advantage over bone. Wood might also be worth considering, though you'd have to treat the "needles" as disposable. I think we alll know that splinters can pierce skin :(
Never encountered porcupine quills myself, not being on a continent that has such. I can tell you that boar bristles are used as needles for leatherwork, but that's for drawing a thread through a ready-prepared hole. I doubt if they'd have the strength to pierce skin.
On the whole, I like the wood idea myself, with the choice of tree having its own significance to the magical effect.
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